The anisotropic Kerr nonlinear refractive index of the beta-barium borate (\beta-BaB2O4) nonlinear crystal

We study the anisotropic nature of the Kerr nonlinear response in a beta-barium borate (\beta-BaB2O4, BBO) nonlinear crystal. The focus is on determining the relevant $\chi^{(3)}$ cubic tensor components that affect interaction of type I cascaded second-harmonic generation. Various experiments in the literature are analyzed and we correct the data from some of the experiments for contributions from cascading as well as for updated material parameters. We find that the Kerr nonlinear tensor component responsible for self-phase modulation in cascading is considerably larger than what has been used to date. We evaluate the impact of using such a cubic anisotropic response in ultrafast cascading experiments.Comment: Updated version, comments on experiments from the literature welcom

Breathing dissipative solitons in optical microresonators

Dissipative solitons are self-localized structures resulting from a double balance between dispersion and nonlinearity as well as dissipation and a driving force. They occur in a wide variety of fields ranging from optics, hydrodynamics to chemistry and biology. Recently, significant interest has focused on their temporal realization in driven optical microresonators, known as dissipative Kerr solitons. They provide access to coherent, chip-scale optical frequency combs, which have already been employed in optical metrology, data communication and spectroscopy. Such Kerr resonator systems can exhibit numerous localized intracavity patterns and provide rich insights into nonlinear dynamics. A particular class of solutions consists of breathing dissipative solitons, representing pulses with oscillating amplitude and duration, for which no comprehensive understanding has been presented to date. Here, we observe and study single and multiple breathing dissipative solitons in two different microresonator platforms: crystalline $\mathrm{MgF_2}$ resonator and $\mathrm{Si_3N_4}$ integrated microring. We report a deterministic route to access the breathing state, which allowed for a detailed exploration of the breathing dynamics. In particular, we establish the link between the breathing frequency and two system control parameters - effective pump laser detuning and pump power. Using a fast detection, we present a direct observation of the spatiotemporal dynamics of individual solitons, revealing irregular oscillations and switching. An understanding of breathing solitons is not only of fundamental interest concerning nonlinear systems close to critical transition, but also relevant for applications to prevent breather-induced instabilities in soliton-based frequency combs.Comment: 10 pages, 4 figure

Detuning-dependent Properties and Dispersion-induced Instabilities of Temporal Dissipative Kerr Solitons in Optical Microresonators

Temporal-dissipative Kerr solitons are self-localized light pulses sustained in driven nonlinear optical resonators. Their realization in microresonators has enabled compact sources of coherent optical frequency combs as well as the study of dissipative solitons. A key parameter of their dynamics is the effective-detuning of the pump laser to the thermally- and Kerr-shifted cavity resonance. Together with the free spectral range and dispersion, it governs the soliton-pulse duration, as predicted by an approximate analytical solution of the Lugiato-Lefever equation. Yet, a precise experimental verification of this relation was lacking so far. Here, by measuring and controlling the effective-detuning, we establish a new way of stabilizing solitons in microresonators and demonstrate that the measured relation linking soliton width and detuning deviates by less than 1 % from the approximate expression, validating its excellent predictive power. Furthermore, a detuning-dependent enhancement of specific comb lines is revealed, due to linear couplings between mode-families. They cause deviations from the predicted comb power evolution, and induce a detuning-dependent soliton recoil that modifies the pulse repetition-rate, explaining its unexpected dependence on laser-detuning. Finally, we observe that detuning-dependent mode-crossings can destabilize the soliton, leading to an unpredicted soliton breathing regime (oscillations of the pulse) that occurs in a normally-stable regime. Our results test the approximate analytical solutions with an unprecedented degree of accuracy and provide new insights into dissipative-soliton dynamics.Comment: Updated funding acknowledgement

Generalized Nonlinear Wave Equation in Frequency Domain

We interpret the forward Maxwell equation with up to third order induced polarizations and get so called nonlinear wave equation in frequency domain (NWEF), which is based on Maxwell wave equation and using slowly varying spectral amplitude approximation. The NWEF is generalized in concept as it directly describes the electric field dynamics rather than the envelope dynamics and because it concludes most current-interested nonlinear processes such as three-wave mixing, four-wave-mixing and material Raman effects. We give two sets of NWEF, one is a 1+1D equation describing the (approximated) planar wave propagation in nonlinear bulk material and the other corresponds to the propagation in a waveguide structure.Comment: Equation Derivation

Soliton-induced nonlocal resonances observed through high-intensity tunable spectrally compressed second-harmonic peaks

Experimental data of femtosecond thick-crystal second-harmonic generation shows that when tuning away from phase matching, a dominating narrow spectral peak appears in the second harmonic that can be tuned over 100's of nm by changing the phase-mismatch parameter. Traditional theory explains this as phase matching between a sideband in the broadband pump to its second-harmonic. However, our experiment is conducted under high input intensities and instead shows excellent quantitative agreement with a nonlocal theory describing cascaded quadratic nonlinearities. This theory explains the detuned peak as a nonlocal resonance that arises due to phase-matching between the pump and a detuned second-harmonic frequency, but where in contrast to the traditional theory the pump is assumed dispersion-free. As a soliton is inherently dispersion-free, the agreement between our experiment and the nonlocal theory indirectly proves that we have observed a soliton-induced nonlocal resonance. The soliton exists in the self-defocusing regime of the cascaded nonlinear interaction and in the normal dispersion regime of the crystal, and needs high input intensities to become excited.Comment: submitted, revised versio

Soliton compression to few-cycle pulses with a high quality factor by engineering cascaded quadratic nonlinearities

We propose an efficient approach to improve few-cycle soliton compression with cascaded quadratic nonlinearities by using an engineered multi-section structure of the nonlinear crystal. By exploiting engineering of the cascaded quadratic nonlinearities, in each section soliton compression with a low effective order is realized, and high-quality few-cycle pulses with large compression factors are feasible. Each subsequent section is designed so that the compressed pulse exiting the previous section experiences an overall effective self-defocusing cubic nonlinearity corresponding to a modest soliton order, which is kept larger than unity to ensure further compression. This is done by increasing the cascaded quadratic nonlinearity in the new section with an engineered reduced residual phase mismatch. The low soliton orders in each section ensure excellent pulse quality and high efficiency. Numerical results show that compressed pulses with less than three-cycle duration can be achieved even when the compression factor is very large, and in contrast to standard soliton compression, these compressed pulses have minimal pedestal and high quality factor

Nonlinear wave equation in frequency domain: accurate modeling of ultrafast interaction in anisotropic nonlinear media

We interpret the purely spectral forward Maxwell equation with up to 3${^{\rm rd}}$ order induced polarizations for pulse propagation and interactions in quadratic nonlinear crystals. The interpreted equation, also named nonlinear wave equation in frequency domain, includes both quadratic and cubic nonlinearities, delayed Raman effects and anisotropic nonlinearities. The full potential of this wave equation is demonstrated by investigating simulations of solitons generated in the process of ultrafast cascaded second-harmonic generation. We show that a balance in the soliton delay can be achieved due to competition between self-steepening, Raman effects and self-steepening-like effects from cascading originating in the group-velocity mismatch between the pump and second harmonic. We analyze the first-order contributions, and show that this balance can be broken to create fast or slow pulses. Through further simulations we demonstrate few-cycle compressed solitons in extremely short crystals, where spectral phenomena such as blue/red shifting, non-stationary radiation in accordance with the non-local phase matching condition and dispersive-wave generation are observed and marked, which help improving the experimental knowledge of cascading nonlinear soliton pulse compression